Transducers for In-pile Ultrasonic Measurements of Fuels and Materials Evolution

Principal Investigator
Name:
Bernhard Tittmann
Email:
[email protected]
Phone:
(208) 526-6918
Team Members:
Name: Institution: Expertise: Status:
Joy Rempe INL - Idaho National Laboratory Using expertise obtained from her role as lead for in-pile instrumentation development and deployment for multiple Department of Energy programs desiring ultrasonics sensors [e.g., the Advanced Test Reactor National Scientific User Facility (ATR NSUF) and the Fuel Cycle Research and Development (FCR&D) programs], Dr. Rempe will help guide the proposed research effort. She will assist by providing insights related to the desired fluence levels for in-pile instrumentation and the types of sensors requiring ultrasonic transducers. Faculty
Leonard Bond Pacific Northwest National Laboratory Using expertise developed as PI for the ARC – ultrasonic Under Sodium Viewing and inspection technologies project, and other studies involving ultrasonic transducers in harsh environments, Dr. Bond will help guide the project, with a focus on aspects of transducer design. He will also provide access to PNNL expertise in transducer design, ultrasonic measurement system design, data analysis and PIE activities Faculty
Experiment Details:
Experiment Title:
Transducers for In-pile Ultrasonic Measurements of Fuels and Materials Evolution)
Abstract
Current generation light water reactors (LWRs), sodium cooled fast reactors (SFRs), small modular reactors (SMRs), of various types, and potentially next generation nuclear plants (NGNPs) all provide harsh environments in and near the core that can severely test material performance, and limit their operational life. As a result of this several Department of Energy Office of Nuclear Energy (DOE-NE) research programs require that the long duration radiation performance of fuels and materials be demonstrated. Such demonstrations in a Material and Test Reactor (MTR) require enhanced instrumentation to detect microstructural changes under the irradiation conditions with unprecedented accuracy and resolution. Recent work supported by DOE?s Advanced Reactor Concepts (ARC) program has been investigating ultrasonic transducers for both under sodium viewing and in-service inspection measurements near the core for fast spectrum reactors. In DOE-NE?s Fuel Cycle Research and Development (FCR&D) program, ultrasonics-based technology was identified as a key approach that should be pursued to obtain the high-fidelity, high-accuracy data required to characterize the behavior and performance of new candidate fuels and structural materials during irradiation testing. Several DOE-NE programs are in the design phase for ultrasonic sensors for in-pile applications; however, these programs are severely limited by the lack of existing knowledge of ultrasonic transducer durability under irradiation conditions. It is therefore proposed that PSU and collaborators assess the performance of common ultrasonic transducer materials (i.e., piezoelectric and magnetostrictive materials) exposed to the high radiation fields for long durations. This test would include both instrumented lead testing to assess the dynamic and transient behavior of the transducer while in-situ as well as post irradiation evaluation to determine sensor material property changes after extended exposures.The proposed research will be completed in five stages: (1) Selection of candidate sensor materials as well as optimization of test assembly parameters. PSU has had longstanding experience in transducer design for harsh environments and is currently designing high temperature transducers for the Intermediate Heat Exchanger in the gas reactor proposed for the next generation nuclear power plant and has had experience testing at the PSU Breazeale Nuclear Reactor. (2) High temperature benchmark testing: will assess the temperature dependent behavior of the sensor materials as a benchmark for the ATR testing. (3) ATR Testing: will be performed to assess sensor degradation by pulse-echo and impedance measurements. (4) Post-Irradiation Evaluation: system components will be inspected at the MFC hot cells to access sensor material property changes. (5) Synthesis: acquired data will be synthesized to assess sensor behavior.The proposed real-time instrumented lead test performed in this ATR NSUF irradiation will provide real-time data related to magnetostrictive and piezoelectric transducer survivability during irradiation testing. This data facilitate the development of transducers for a variety of in-pile measurements in MTRs, including sensors to perform temperature measurements and characterize the properties of fuels and structural materials of interest to several DOE-NE programs. This work is a necessary step for DOE-NE programs to design in-pile sensors necessary for evaluating the long duration performance of fuel and structural materials.
Book / Journal Publications

"Progress towards developing neutron tolerant magnetostrictive and piezoelectric transducers" Brian Reinhardt, Bernhard Tittmann, Joy Rempe, Joshua Daw, Gordon Kohse, David Carpenter, Michael Ames, Yakov Ostrovsky, Pradeep Ramuhalli, Robert Montgomery, Hualte Chien, Bernard Wernsman, AIP Conference Proceedings 1650 2015 1512-1520 Link

"Nuclear Radiation Tolerance of Single Crystal Aluminum Nitride Ultrasonic Transducer" Bernhard Tittmann, Brian Reinhardt, Andrew Suprock, Physics Procedia 70 2015 609-613 Link

"Irradiation Testing of Ultrasonic Transducers" Joshua Daw, Gordon Kohse, Joe Palmer, Pradeep Ramuhalli, Brian Reinhardt, Joy Rempe, Bernhard Tittmann, Robert Montgomery, Jean-Francois Villard, H. T. Chien, ANIMMA 2013 Special Edition, IEEE Transactions on Nuclear Science 61 2013 1-7 Link

"Updated Results of Ultrasonic Transducer Irradiation Test" Joshua Daw, Gordon Kohse, Joe Palmer, Brian Reinhardt, Joy Rempe, Pradeep Ramuhalli, Paul Keller, Robert Montgomery, Hual-Te Chien, Bernhard Tittmann, Jean-Francois Villard, ANIMMA - Institute of Electrical and Electronics Engineers 2015 Link

"Irradiation Testing of Piezoelectric (Aluminum Nitride, Zinc Oxide, and Bismuth Titanate) and Magnetostrictive Sensors (Remendur and Galfenol)" Joshua Daw, Brian Reinhardt, Bernhard Tittmann, IEEE Transactions on Nuclear Science 65 2018 Link

"Effect of sintering temperature on adhesion of spray-on piezoelectric transducers" , Journal of Sensors and Senor Systems 5 2016 113-123

"Testing piezoelectric sensors in a nuclear reactor environment" Brian Reinhardt, Andy Suprock, Bernhard Tittmann, AIP Conference Proceedings 1806 2017 Link

"High Temperature (>500C) Ultrasonic Transducers: An Experimental Comparison Among Three Candidate Piezoelectric Materials" Bernhard Tittmann, IEEE Transactions on Ultrasonics, Ferroelectrics and Frequency Control 60 2013 1010-1015 Link

Conference Publications

"Irradiation Testing of Ultrasonic Transducers" Joshua Daw, Gordon Kohse, Joe Palmer, Pradeep Ramuhalli, Brian Reinhardt, Joy Rempe, Bernhard Tittmann, 2013 Conference on Advancements in Nuclear Instrumentation, Measurements Methods (ANIMMA 2013) June 23-27, (2013)